Uranium elimination and its retrieval from waste water or any other water sources, by the means of reducing biological risks and Uranium recycling to the main environment cycle, possess a high level of value. In this research, by producing Polymeric Nano-Absorbent, the possibility of Uranium Segregation from water such as Nuclear Center waste water will be discussed. For this, Nano-Fibre Polycarbonate was produced by adopting the modern technology of Forcespinning. SEM images illustrated that the fibre diameter is within the allowed Nano limitation. In order to reclaim the surface of the net polycarbonate, two procedures of Bonding and Making Nano-Fibre Composite were considered. In Bonding, Glycidyl Methacrylate (GMA) was bonded on the surface of the Polycarbonate using radiation process. For this, the Nano-Fibre Polycarbonate with the doze of 200 kGy was radiated. After that, it was kept in the lotion of Glycidyl Methacrylate (GMA) 10% and Methanol, in 40 o C for 8 hours. Then, to convert the produced epoxies groups by Glycidyl Methacrylate (GMA), to Nitrile groups, the Polycarbonate was held in lotion of 0.245 mole Imino di-propionitrile and Ethanol in 80 o C for 72 hours. Infrared Spectroscopy was the testimony of joined Nitrile Groups to the surface of Polycarbonate. The remained reclaimed Polycarbonate in the lotion, at the end of the reaction was dissolved and decreased. Subsequently, it required modifying in some parameters such as the amount of radiation and the solvents used in the reaction. However, because of the cost matters, time constraint and technological limitation, re-radiation and re-producing the sample in order to achieve the reclaimed form of the lotion, were not possible. So, this procedure was ignored and the second reclaiming procedure of providing the Polycarbonate and Copolymertyrene – Acrylonitrile composites was considered. SEM images of the Composite Fibres illustrated that the fibre diameter is within the allowed Nano limitation. As the Styrene Acrylonitrile includes Nitrile Groups, it is more convenient, rather than Uranium, to be bonded to the surface of Polycarbonate and promote its absorb ability. After the production of the Nano-Fibre Composites of Polycarbonate and Styrene Acrylonitrile, these Nano-Fibre were put in the lotion of Amin Hydroxyl 10% in 80 o C for 72 hours to convert the Nitrile Groups to Amidoxime groups. By using Infrared Spectroscopy, this conversion was proved. Then, prior to carrying out the Absorption Test, in order to develop the effectiveness of the produced Nano-Absorbent material, they were kept in the alkaline lotion of Sodium hydroxide 2.5% in 80 o C for 3 hours. Then, in order to achieve the produced Nano-Abosbent material, determined amounts of these absorbents were kept and stirred in a lotion containing specified viscosity Uranium for 24 hours. The amount of absorption made by the absorbent before the process and after it, were measured and the ability of absorb of the absorbent was determined. The value was 38.5 milligram in respect to the existence of 1 gram absorbent. In order to achieve the optimum PH, the performance of the absorbent was measured in PH=3 to PH=7. The best effectiveness of the absorbent was observed in PH=4. Consequently, the resorption of this absorbent was measured in 1 mole lotion of Na 2 CO 3 and H 2 O 2 , which was 90%. Keywords Nanofibers, Forcespinning, Graft, Adsorbent, Uranium